Ultrafast interaction of the angular momentum of photons with spins in the metallic amorphous alloy GdFeCo.

Ultrashort laser pulses have been used to study the effect of circularly polarized light on spins in the ferrimagnetic metal GdFeCo. By turning the sample into a multidomain state and thereby suppressing the observation of the heating effect of light, we have been able to demonstrate an ultrafast nonthermal excitation of spin waves with a phase that depends on the angular momentum of the photons. These results demonstrate the possibility of ultrafast coherent control of the magnetization in this metallic system.